Published April 8, 2020 | Version v1
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Cascade trifluoromethylthiolation and cyclization of <i>N</i>-[(3-aryl)propioloyl]indoles

  • 1. Donghua University
  • 2. Shanghai Institute of Organic Chemistry

Description

A cascade oxidative trifluoromethylthiolation and cyclization of N -[(3-aryl)propioloyl]indoles with AgSCF 3 is described. This protocol allows for the synthesis of novel bis(trifluoromethylthiolated) or trifluoromethylthiolated pyrrolo[1,2- a ]indol-3-ones in moderate to good yields. Mechanistic investigations indicated that radical processes were probably involved in these transformations.

⚠️ This is an automatic machine translation with an accuracy of 90-95%

Translated Description (Arabic)

يوصف تفاعل ثلاثي فلورو ميثيل ثيول تتالي وتدوير إنديولات N -[(3 -آريل) بروبيولويل] مع AgSCF 3. يسمح هذا البروتوكول بتوليف مكرر جديد (ثلاثي فلورو ميثيل ثيولاتيد) أو ثلاثي فلورو ميثيل ثيولاتيد بيرولو[1،2 - a ]إندول-3 -واحد في غلة معتدلة إلى جيدة. أشارت التحقيقات الميكانيكية إلى أن العمليات الجذرية ربما كانت متورطة في هذه التحولات.

Translated Description (French)

Une trifluorométhylthiolation oxydative en cascade et une cyclisation de N -[(3-aryl) propioloyl]indoles avec AgSCF 3 sont décrites. Ce protocole permet la synthèse de nouvelles pyrrolo[1,2- a] indol-3-ones bis(trifluorométhylthiolées) ou trifluorométhylthiolées avec des rendements modérés à bons. Des investigations mécanistiques ont indiqué que des processus radicaux étaient probablement impliqués dans ces transformations.

Translated Description (Spanish)

Se describe una trifluorometiltiolación oxidativa en cascada y ciclación de N -[(3-aril) propiloil]indoles con AgSCF 3. Este protocolo permite la síntesis de nuevas pirrolo[1,2-a] indol-3-onas bis(trifluorometiltioladas) o trifluorometiltioladas con rendimientos moderados a buenos. Las investigaciones mecanicistas indicaron que los procesos radicales probablemente estaban involucrados en estas transformaciones.

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Additional details

Additional titles

Translated title (Arabic)
تتالي ثلاثي فلورو <i>ميثيل ثيول وتدوير إن</i>-[(3 -أريل)بروبيولويل]إندولز
Translated title (French)
Trifluorométhylthiolation en cascade et cyclisation des <i>N</i>-[(3-aryl)propioloyl]indoles
Translated title (Spanish)
Trifluorometiltiolación en cascada y ciclación de <i>N-</i> [(3-aril)propiloil]indoles

Identifiers

Other
https://openalex.org/W3015491700
DOI
10.3762/bjoc.16.62

GreSIS Basics Section

Is Global South Knowledge
Yes
Country
China

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